To transfer playlist to iTunes Library from iPod, you may try to use TunesGo. It allows you to transfer music, playlist and movies from iPod to iTunes Library. The most amazing function of this music transfer software is that it supports not only iPhone/iPad/iPod, but also other Android phone model like Samsung, HTC, LG, Sony, and more (Android 2.1 ~ Android 5.0).
To copy playlist between iPod and iTunes, please download TunesGo on your computer, connect iPod to PC with a USB cable. Make sure that iTunes is well installed on PC. If you're using Mac, you can also download TunesGo for Mac.
Download TunesGo on your computer, install it and launch it on PC. After that, connect your iPod to computer via USB cable and move on.
Step 2 Export iPod touch 5 playlist to iTunes Library
You will see the below window showing the iPod touch 5 and the detail info as well. In the interface, choose the playlist under iPod list. Then, right click the playlist and click "Export to iTunes".
Note: You can also transfer playlist with this software. And different Android OS are supported, including Android 2.1 to Android 5.0.
Now, you can check your iTunes Library to see if the playlist is transferred. You may also transfer music files from iPod to computer. transfer music files from iPod to computer. Click and download TunesGo below. You can also see how to put music from iPod to iTunes.